I'd go with probably "Goodbye to Bloo" partially because of all the great inside jokes to the earlier episodes. Just a great way to send off the series.
To me it wasn't any particular episode that stands out as much as moments in the episodes. For example I can't think of one that I was rolling over laughing the whole episode but I can sure tell you the first time I saw the chase in the junkyard in the pilot where the shot pans out and then Pac Man music comes on killed me, and still does almost every time.
Coco just in general also hit me as strikingly hilarious.
I guess a couple special mentions for hilarity is "Mac Daddy" and "Cheese a Gogo" (mainly thanks to a very much inabriated Eduardo).
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